Published April 10, 2024 | Version v1
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Generation and Propagation of Flexoelectricity-Induced Solitons in Nematic Liquid Crystals

  • 1. University of Chicago
  • 2. Indian Institute of Technology
  • 3. Cornell University

Description

Solitons in nematic liquid crystals facilitate the rapid transport and sensing in microfluidic systems. Little is known about the elementary conditions needed to create solitons in nematic materials. In this study, we apply a combination of theory, computational simulations, and experiments to examine the formation and propagation of solitary waves, or "solitons", in nematic liquid crystals under the influence of an alternating current (AC) electric field. We find that these solitary waves exhibit "butterfly"-like or "bullet"-like structures that travel in the direction perpendicular to the applied electric field. Such structures propagate over long distances without losing their initial shape. The theoretical framework adopted here helps identify several key factors leading to the formation of solitons in the absence of electrostatic interactions. These factors include surface irregularities, flexoelectric polarization, unequal elastic constants, and negative anisotropic dielectric permittivity. The results of simulations are shown to be in good agreement with our own experimental observations, serving to establish the validity of the theoretical concepts and ideas advanced in this work.

Data availability

The data that support the findings of the study are available from the corresponding author upon reasonable request.

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Additional details

Identifiers

DOI
10.1021/acsnano.3c10800
Other
oai:uchicago.tind.io:13339

Funding

U.S. Department of Energy
DESC0019762

UChicago Information

Division(s)
Pritzker School of Molecular Engineering