Published March 4, 2016
| Version v1
Journal article
Open
Origin of uranium isotope variations in early solar nebula condensates
Description
High-temperature condensates found in meteorites display uranium isotopic variations (235U/238U) that complicate dating the solar system's formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide 247Cm (t1/2 = 15.6 My) into 235U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of 235U reaching ∼+6% relative to average solar system composition, which can only be due to the decay of 247Cm. This allows us to constrain the 247Cm/235U ratio at solar system formation to (7.0 ± 1.6) × 10-5. This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture.
Data availability
All data needed to evaluate the conclusions in the paper are present in the paper and/or the Supplementary Materials. Additional data are available from the authors upon request. This is Origins Lab contribution number 91.Files
sciadv.1501400.pdf
Files
(8.7 MB)
| Name | Size | Download all |
|---|---|---|
|
Supplementary materials md5:5af3cde5686f36e7aeaf5938bab2ea17 |
7.1 MB | Preview Download |
|
Article md5:1e42106d9ef8cbb445c291d54f40f833 |
1.6 MB | Preview Download |
Additional details
Identifiers
- DOI
- 10.1126/sciadv.1501400
- Other
- oai:uchicago.tind.io:11002
Related works
- Is supplement to
- https://doi.org/10.1126/sciadv.1602881 (URL)
Funding
- National Aeronautics and Space Administration
- NNX14AK09G
- National Aeronautics and Space Administration
- OJ-30381-0036A
- National Aeronautics and Space Administration
- NNX15AJ25G
- National Science Foundation
- EAR144495
- National Science Foundation
- EAR150259
- National Aeronautics and Space Administration
- NNX13AE73G