Published March 4, 2016 | Version v1
Journal article Open

Origin of uranium isotope variations in early solar nebula condensates

  • 1. University of Chicago

Description

High-temperature condensates found in meteorites display uranium isotopic variations (235U/238U) that complicate dating the solar system's formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide 247Cm (t1/2 = 15.6 My) into 235U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of 235U reaching ∼+6% relative to average solar system composition, which can only be due to the decay of 247Cm. This allows us to constrain the 247Cm/235U ratio at solar system formation to (7.0 ± 1.6) × 10-5. This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture.

Data availability

All data needed to evaluate the conclusions in the paper are present in the paper and/or the Supplementary Materials. Additional data are available from the authors upon request. This is Origins Lab contribution number 91.

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Additional details

Identifiers

DOI
10.1126/sciadv.1501400
Other
oai:uchicago.tind.io:11002

Related works

Funding

National Aeronautics and Space Administration
NNX14AK09G
National Aeronautics and Space Administration
OJ-30381-0036A
National Aeronautics and Space Administration
NNX15AJ25G
National Science Foundation
EAR144495
National Science Foundation
EAR150259
National Aeronautics and Space Administration
NNX13AE73G

UChicago Information

Division(s)
Physical Sciences Division
Department(s)
Enrico Fermi Institute, Geophysical Sciences